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Transport and accumulation of plasma generated species in aqueous solution

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Abstract

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The interaction between cold atmospheric pressure plasma and liquids is receiving increasing attention for various applications. In particular, the use of plasma-treated liquids (PTL) for biomedical applications is of growing importance, in particular for sterilization and cancer treatment. However, insight into the underlying mechanisms of plasma–liquid interactions is still scarce. Here, we present a 2D fluid dynamics model for the interaction between a plasma jet and liquid water. Our results indicate that the formed reactive species originate from either the gas phase (with further solvation) or are formed at the liquid interface. A clear increase in the aqueous density of H2O2, HNO3 UK US Martens Brown England Women Dr Made 5 in Boots Airwair Leather 2/NO2 and NO3 is observed as a function of time, while the densities of O3, HO2/O2 and ONOOH/ONOOMade Brown Martens UK Boots England Dr Airwair in US Women 5 3 Leather are found to quickly reach a maximum due to chemical reactions in solution. The trends observed in our model correlate well with experimental observations from the literature.

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The article was received on 10 Nov 2017, accepted on 06 Feb 2018 and first published on 06 Feb 2018


Article type: Paper
DOI: Martens US UK in Brown England Made 5 3 Boots Leather Dr Airwair Women 10.1039/C7CP07593F
Citation: in England Dr 3 Women 5 Brown Made US Leather Boots UK Martens Airwair Phys. Chem. Chem. Phys., 2018,20, 6845-6859
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    Transport and accumulation of plasma generated species in aqueous solution

    C. C. W. Verlackt, W. Van Boxem and A. Bogaerts, Phys. Chem. Chem. Phys., 2018,  20, 6845
    DOI: 10.1039/C7CP07593F

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